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泉州湾表层沉积物中多环芳烃的含量 分布特征及污染来源

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庄婉娥, 汪厦霞, 姚文松, 杨琳, 宋希坤, 弓振斌. 泉州湾表层沉积物中多环芳烃的含量 分布特征及污染来源[J]. 环境化学, 2011, 30(5): 928-934.
引用本文: 庄婉娥, 汪厦霞, 姚文松, 杨琳, 宋希坤, 弓振斌. 泉州湾表层沉积物中多环芳烃的含量 分布特征及污染来源[J]. 环境化学, 2011, 30(5): 928-934.
shu
ZHUANG Wane, WANG Xiaxia, YAO Wensong, YANG Lin, SONG Xikun, GONG Zhenbin. DISTRIBUTION AND SOURCE OF POLYCYCLIC AROMATIC HYDROCARBONS IN THE SURFACE SEDIMENTS OF QUANZHOU BAY, CHINA[J]. Environmental Chemistry, 2011, 30(5): 928-934.
Citation: ZHUANG Wane, WANG Xiaxia, YAO Wensong, YANG Lin, SONG Xikun, GONG Zhenbin. DISTRIBUTION AND SOURCE OF POLYCYCLIC AROMATIC HYDROCARBONS IN THE SURFACE SEDIMENTS OF QUANZHOU BAY, CHINA[J]. Environmental Chemistry, 2011, 30(5): 928-934.
shu

泉州湾表层沉积物中多环芳烃的含量 分布特征及污染来源

  • 1.

    厦门大学近海海洋环境科学国家重点实验室, 厦门, 361005;

  • 2.

    厦门大学海洋与环境学院, 厦门, 361005;

  • 3.

    福建省海洋环境与渔业资源监测中心, 福州, 350003

  • 基金项目:

    海洋公益性行业科研专项(No.200705029)资助.

DISTRIBUTION AND SOURCE OF POLYCYCLIC AROMATIC HYDROCARBONS IN THE SURFACE SEDIMENTS OF QUANZHOU BAY, CHINA

  • 1.

    State Key Laboratory of Marine Environmental Science, Xiamen University, Xiamen, 361005, China;

  • 2.

    College of Oceanography and Environmental Science, Xiamen University, Xiamen, 361005, China;

  • 3.

    Monitoring Center of Marine Environment and Fishery Resource, Fujian Province, Fuzhou, 350003, China

  • Fund Project:

  • 摘要: 采用气相色谱-质谱联用(GC-MS)方法,对泉州湾表层沉积物中16种优先控制多环芳烃(PAHs)进行定量分析,采用LMW/HMW、BaA/(BaA+Chr)、InP/(InP+BgP)、Ppi等特定比值对PAHs来源进行分析.结果表明,沉积物中PAHs的总含量在182.8—721.1 ng·g-1之间,以3—5环为主;PAHs在表层沉积物中的含量分布总体呈现为泉州湾南岸高于北岸、内湾高于外湾;沉积物中PAHs主要来自高温不完全燃烧.与国内外其它海域相比,泉州湾PAHs处于中等污染水平,该区域表层沉积物中的PAHs对生物不存在明显的毒性效应,但具有潜在的毒副作用.
    Abstract: The concentrations of 16 polycyclic aromatic hydrocarbons (PAHs) in the surface sediments of Quanzhou Bay, China, were measured with gas chromatography-mass spectrometry (GC-MS). Source-specific PAHs indexes, including LMW/HMW, BaA/(BaA+Chr), InP/(InP+BgP) and Ppi, were used to identify the potential sources of PAHs in this region. The total contents of PAHs in the sediments were in the range of 182.8—721.1 ng·g-1, which were dominated by PAHs of 3—5 rings. The concentration of PAHs in the Bay was higher in the south bank than in the north bank, and higher in the inner bay than in the outer bay as well. The indexes of source identification indicated that incomplete combustion was the dominant source of PAHs in this study. The pollution of PAHs in the Bay was moderate compared with other regions in the world. PAHs in the surface sediments in this area would not cause remarkably negative effects on marine organisms, but potential negative effects should not be overlooked.
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  • [1] Callahan M A, Slimak M W, Gabelc N W, et al. Water-related environmental fate of 129 priority pollutants . EPA-440/4-79-029
    [2] Doong R, Lin Y. Characterization and distribution of polycyclic aromatic hydrocarbon contaminations in surface sediments and water from Gao-ping River, Taiwan [J]. Water Research, 2004, 38(7): 1733-1744
    [3] 麦碧娴, 林峥, 张干,等. 珠江三角洲河流和珠江口表层沉积物中有机污染物研究——多环芳烃和有机氯农药的分布及特征 [J]. 环境科学学报, 2000, 20(2): 192-197
    [4] Yu R, Yuan X, Zhao Y, et al. Heavy metal pollution in intertidal sediments from Quanzhou Bay, China [J]. Journal of Environmental Sciences, 2008, 20(6): 664-669
    [5] 袁建军, 谢嘉华. 泉州湾近岸海域水质状况调查与评价 [J]. 台湾海峡, 2003, 22(1): 14-18
    [6] Gong X, Qi S, Wang Y, et al. Historical contamination and sources of organochlorine pesticides in sediment cores from Quanzhou Bay, Southeast China [J]. Marine Pollution Bulletin, 2007, 54(9): 1434-1440
    [7] 林峥, 麦碧娴, 张干,等. 沉积物中多环芳烃和有机氯农药定量分析的质量保证和质量控制 [J]. 环境化学, 1999, 18(2): 115-121
    [8] 吴永宁, 江桂斌. 重要有机污染物痕量与超痕量检测技术 [M]. 北京: 化学工业出版社, 2007: 369
    [9] Fang M, Hsieh P, Ko F, et al. Sources and distribution of polycyclic aromatic hydrocarbons in the sediments of Kaoping river and submarine canyon system, Taiwan [J]. Marine Pollution Bulletin, 2007, 54(8): 1179-1189
    [10] Chen Y, Zhu L, Zhou R. Characterization and distribution of polycyclic aromatic hydrocarbon in surface water and sediment from Qiantang River, China [J]. Journal of Hazardous Materials, 2007, 141(1): 148-155
    [11] 杨敏, 倪余文, 苏凡,等. 辽河沉积物中多环芳烃的污染水平与特征 [J]. 环境化学, 2007, 26(2): 217-220
    [12] Zhu L, Cai X, Wang J. PAHs in aquatic sediment in Hangzhou, China: analytical methods, pollution pattern, risk assessment and sources [J]. Journal of Environmental Sciences-China, 2005, 17(5): 748-755
    [13] Zhang Z, Hong H, Zhou J, et al. Phase association of polycyclic aromatic hydrocarbons in the Minjiang River estuary, China [J]. Science of The Total Environment, 2004, 323(1-3): 71-86
    [14] Maskaoui K, Zhou J, Hong H, et al. Contamination by polycyclic aromatic hydrocarbons in the Jiulong River estuary and Western Xiamen Sea, China [J]. Environmental Pollution, 2002, 118(1): 109-122
    [15] Men B, He M, Tan L, et al. Distributions of polycyclic aromatic hydrocarbons in the Daliao River Estuary of Liaodong Bay, Bohai Sea (China) [J]. Marine Pollution Bulletin, 2009, 58(6): 818-826
    [16] Hong H, Xu L, Zhang L, et al. Environmental fate and chemistry of organic pollutants in the sediments of Xiamen and Victoria Harbours [J]. Marine Pollution Bulletin, 1995, 31(4-12): 229-236
    [17] Pereira W, Hostettler F, Rapp J. Distribution and fate of chlorinated insecticides, biomarkers and polycyclic aromatic hydrocarbons in sediments along a contamination gradient from a point source in San-Francisco Bay [J]. Marine Environmental Research, 1996, 41(3): 299-314
    [18] Viguri J, Verde J, Irabien A. Environmental assessment of polycyclic aromatic hydrocarbon (PAHs) in surface sediments of the Santander Bay, Northern Spain [J]. Chemosphere, 2002, 48(2): 157-165
    [19] Yan W, Chi J, Wang Z, et al. Spatial and temporal distribution of polycyclic aromatic hydrocarbons (PAHs) in sediments from Daya Bay, South China [J]. Environmental Pollution, 2009, 157(6): 1823-1830
    [20] Mostafa A, Wade T, Sweet S, et al. Distribution and characteristics of polycyclic aromatic hydrocarbons (PAHs) in sediments of Hadhramout coastal area, Gulf of Aden, Yemen [J]. Journal of Marine Systems, 2009, 78(1): 1-8
    [21] Baumard P, Budzinski H, Garrigues P. Polycyclic aromatic hydrocarbons in sediments and mussels of the western Mediterranean Sea [J]. Environmental Toxicology and Chemistry, 1998, 17(5): 765-776
    [22] Long E, MacDonald D, Smith S, et al. Incidence of adverse biological effects within ranges of chemical concentrations in marine and estuarine sediments [J]. Environmental Management, 1995, 19(1): 81-97
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  • 收稿日期:  2010-05-17
庄婉娥, 汪厦霞, 姚文松, 杨琳, 宋希坤, 弓振斌. 泉州湾表层沉积物中多环芳烃的含量 分布特征及污染来源[J]. 环境化学, 2011, 30(5): 928-934.
引用本文: 庄婉娥, 汪厦霞, 姚文松, 杨琳, 宋希坤, 弓振斌. 泉州湾表层沉积物中多环芳烃的含量 分布特征及污染来源[J]. 环境化学, 2011, 30(5): 928-934.
shu
ZHUANG Wane, WANG Xiaxia, YAO Wensong, YANG Lin, SONG Xikun, GONG Zhenbin. DISTRIBUTION AND SOURCE OF POLYCYCLIC AROMATIC HYDROCARBONS IN THE SURFACE SEDIMENTS OF QUANZHOU BAY, CHINA[J]. Environmental Chemistry, 2011, 30(5): 928-934.
Citation: ZHUANG Wane, WANG Xiaxia, YAO Wensong, YANG Lin, SONG Xikun, GONG Zhenbin. DISTRIBUTION AND SOURCE OF POLYCYCLIC AROMATIC HYDROCARBONS IN THE SURFACE SEDIMENTS OF QUANZHOU BAY, CHINA[J]. Environmental Chemistry, 2011, 30(5): 928-934.
shu

泉州湾表层沉积物中多环芳烃的含量 分布特征及污染来源

  • 1.  厦门大学近海海洋环境科学国家重点实验室, 厦门, 361005;
  • 2.  厦门大学海洋与环境学院, 厦门, 361005;
  • 3.  福建省海洋环境与渔业资源监测中心, 福州, 350003
  • 收稿日期:  2010-05-17
基金项目:

海洋公益性行业科研专项(No.200705029)资助.

摘要: 采用气相色谱-质谱联用(GC-MS)方法,对泉州湾表层沉积物中16种优先控制多环芳烃(PAHs)进行定量分析,采用LMW/HMW、BaA/(BaA+Chr)、InP/(InP+BgP)、Ppi等特定比值对PAHs来源进行分析.结果表明,沉积物中PAHs的总含量在182.8—721.1 ng·g-1之间,以3—5环为主;PAHs在表层沉积物中的含量分布总体呈现为泉州湾南岸高于北岸、内湾高于外湾;沉积物中PAHs主要来自高温不完全燃烧.与国内外其它海域相比,泉州湾PAHs处于中等污染水平,该区域表层沉积物中的PAHs对生物不存在明显的毒性效应,但具有潜在的毒副作用.

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