武汉典型下垫面降雨径流PAHs污染特征研究
Investigation on PAHs Characteristics in Runoff of Different Underlying Surfaces in Wuhan
-
摘要: 以武汉城区7类典型下垫面降雨径流中16种多环芳烃(polycyclic aromatic hydrocarbons, PAHs)为主要研究对象，对径流中常规污染物、PAHs浓度、种类差异与来源等进行研究。结果表明，武汉市7类下垫面降雨径流中，在常规污染物方面，沥青路面和水泥路面的污染程度最高，瓦屋面污染程度最低；而在PAHs方面，沥青路面径流∑16PAHs初始浓度最高，2类油毡屋面(工业园和教工宿舍)次之，其他4类下垫面较低。油毡屋面径流PAHs主要由蒽(ANT)和菲(PHE)组成，而沥青路面、水泥路面等其他5类下垫面径流中主要含有PHE、芘(PYR)和荧蒽(FLA)等。油毡屋面(工业园和教工宿舍)、水泥屋面和瓦屋面等4类屋面径流中主要污染物是2～3环PAHs，而沥青路面和水泥路面径流中则以4～6环PAHs为主。Abstract: Rainfall runoff samples were collected at seven typical underlying surfaces in Wuhan City. In this study, the concentrations, species differences and sources of conventional pollutants and 16 PAHs in the runoff were investigated. The results showed that the initial concentration of ∑16PAHs in asphalt pavement runoff was the highest, followed by two types of linoleum roofs (industrial park and teacher dormitory), and the other four underlying surfaces. Meanwhile, the PAHs in the runoff of linoleum roofs were mainly composed of anthracene (ANT) and phenanthrene (PHE), while the PAHs in the runoff of the other five underlying surfaces were predominantly comprised of phenanthrene (PHE), pyrene (PYR), and fluoranthene (FLA), etc. Furthermore, 2～3 ring PAHs were dominant in the runoff of those four roofs (industrial park, teacher dormitory, cement and tile roofs), while 5～6 ring PAHs were major components in the runoff of those two pavements (linoleum and cement).
-
Key words:
- PAHs /
- rainfall runoff /
- urban underlying surface /
- Wuhan
-
-
侯培强,王效科,郑飞翔,等.我国城市面源污染特征的研究现状[J].给水排水, 2009, 35(s1):188-193 Hou P Q, Wang X K, Zheng F X, et al. Research status of urban non-point source pollution characteristics in China[J]. Water & Wastewater Engineering, 2009, 35(s1):188-193(in Chinese)
Gnecco I, Berretta C, Lanza L G, et al. Storm water pollution in the urban environment of Genoa, Italy[J]. Atmospheric Research, 2005, 77(1):60-73 Xu S S, Liu W X, Tao S. Emission of polycyclic aromatic hydrocarbons in China[J]. Environmental Science & Technology, 2006, 40(3):702-708 Brown J N, Peake B M. Sources of heavy metals and polycyclic aromatic hydrocarbons in urban stormwater runoff[J]. Science of the Total Environment, 2006, 359(1/3):145-155 Forster J. Variability of roof runoff quality[J].Water Science & Technology, 1999, 39(5):137-144 欧浪波,胡丹,黄晔,等.北京城区屋面径流中PAHs的初期冲刷效应[J].环境科学, 2011, 32(10):2896-2912 Ou L B, Hu D, Huang Y, et al. First flush analysis of PAHs in roof runoff in Beijing[J]. Environmental Science, 2011, 32(10):2896-2912(in Chinese)
边璐,李田,侯娟. PMF和PCA/MLR法解析上海市高架道路地表径流中多环芳烃的来源[J].环境科学, 2013, 34(10):3840-3846 Bian L, Li T, Hou J. Source apportionment of polycyclic aromatic hydrocarbons using two mathematical models for runoff of the Shanghai elevated inner highway, China[J]. Environmental Science, 2013, 34(10):3840-3846(in Chinese)
Scheeper P T, Houtum J V, Anzion R B, et al. The occupational exposure of dermatology nurses to polycyclic aromatic hydrocarbons-evaluating the effectiveness of better skin protection[J]. Scandinavian Journal of Work Environment & Health, 2009, 35(3):212-221 周婕成.城市降雨径流中多环芳烃的污染特征、源解析及生态风险评价[D].上海:华东师范大学, 2011:65-68 Zhou J C. The pollution characteristics, source identification and ecological risk assessment of PAHs in urban runoff[D]. Shanghai:East China Normal University, 2011:65 -68(in Chinese)
武子澜,杨毅,刘敏,等.城市不同下垫面降雨径流多环芳烃(PAHs)分布及源解析[J].环境科学, 2014, 35(11):4148-4156 Wu Z L, Yang Y, Liu M, et al. Distribution and source apportionment of polycyclic aromatic hydrocarbons (PAHs) in urban rainfall runoff[J]. Environmental Science, 2014, 35(11):4148-4156(in Chinese)
Zhang W, Zhang S C, Wan C, et al. Source diagnostics of polycyclic aromatic hydrocarbons in urban road runoff, dust, rain and canopy through fall[J]. Environmental Pollution, 2008, 153(3):594-601 Murakami M, Nakajima F, Furumai H. Modeling of runoff behavior of particle-bound polycyclic aromatic hydrocarbons (PAHs) from roads and roofs[J]. Water Research, 2004, 38(20):4475-4483 谢继锋,李静静,窦月芹,等.不同下垫面类型对地表径流中多环芳烃污染特征的影响分析[J].环境化学, 2015, 34(4):733-740 Xie J F, Li J J, Dou Y Q, et al. Pollution characteristics of PAHs in urban runoffs on different types of underlying surfaces[J]. Environmental Chemistry, 2015, 34(4):733-740(in Chinese)
Sun Y W, Zhang D, Wang Z W. The potential of using biological nitrogen removal technique for stormwater treatment[J]. Ecological Engineering, 2017, 106:482-495 王浩升.武汉市不同下垫面降雨径流污染特征分析与污染负荷估算[D].武汉:华中科技大学, 2015:56-59 Wang H S. Pollution charactersistics analysis and pollution load estimation in rainfall runoff of different underlying surface in Wuhan City[D]. Wuhan:Huazhong University of Science and Technology, 2015:56 -59(in Chinese)
Halsall C J, Coleman P J, Davis B J, et al. Polycyclic aromatic hydrocarbons in UK urban air[J]. Environmental Science and Technology, 1994, 28(13):2380-2386 Harrison R M, Smith D J T, Luhana L. Source apportionment of atmospheric polycyclic aromatic collected from an urban location in Birmingham, UK[J]. Environmental Science and Technology, 1996, 30(3):825-832 武子澜.城市降雨径流和地表灰尘PAHs赋存迁移及其生态风险评价[D].上海:华东师范大学, 2015:46-52 Wu Z L. The occurrence level, transport and ecological risk assessment of PAHs in urban rainfall runoff and dust[D]. Shanghai:East China Normal University, 2015:46 -52(in Chinese)
胡丹,欧浪波,黄晔,等.北京城区屋面径流中PAHs的污染特征与来源解析[J].生态环境学报, 2010, 19(11):2613-2618 Hu D, Ou L B, Huang Y, et al. Concentration characteristics and source identification of PAHs in urban roof runoff in Beijing[J]. Ecology and Environmental Sciences, 2010, 19(11):2613-2618(in Chinese)
张巍,张树才,岳大攀,等.北京城市道路地表径流中PAHs的污染特征研究[J].环境科学学报, 2008, 28(1):160-167 Zhang W, Zhang S C, Yue D P, et al. Study on PAHs concentrations in urban road runoff in Beijing[J]. Acta Scientiae Circumstantiae, 2008, 28(1):160-167(in Chinese)
Feng C L, Xia X H, Shen Z Y, et al. Distribution and sources of polycyclic aromatic hydrocarbons in Wuhan section of the Yangtze River, China[J]. Environmental Monitoring and Assessment, 2007, 133(1/3):447-458 Boxall A B A, Maltbyl L. The effects of motorway runoff on freshwater ecosystems. 3. Toxicant confirmation[J]. Archives of Environmental Contamination and Toxicology, 1997, 33(1):9-16 刘宪斌,杨文晓,田胜艳,等.曹妃甸和黄骅港近岸海域表层水体中PAHs的分布、来源及风险评价[J].生态毒理学报, 2016, 11(2):742-748 Liu X B, Yang W X, Tian S Y, et al. Distribution, source and ecological risk assessment of polycyclic aromatic hydrocarbons in surface water from the Caofeidian and Huanghuagang, China[J]. Asian Journal of Ecotoxicology, 2016, 11(2):742-748(in Chinese)
Mackay D, Shiu W Y, Ma K C, et al. Handbook of Physical-Chemical Properties and Environmental Fate for Organic Chemicals[M]. 2nd ed. New York:CRC Press, 2006:315-320 Oliver M À. Polycyclic aromatic hydrocarbons in rainwater and surface waters of Lake Maggiore, a subalpine lake in Northern Italy[J]. Chemosphere, 2006, 63(1):116-131 张巍,张树才,万超,等.北京城市道路地表径流及相关介质中多环芳烃的源解析[J].环境科学, 2008, 29(6):1478-1483 Zhang W, Zhang S C, Wan C, et al. PAH sources in road runoff system in Beijing[J]. Environmental Science, 2008, 29(6):1478-1483(in Chinese)
韩景超,毕春娟,陈振楼,等.城市交通干道降雨径流中PAHs的污染特征[J].环境科学学报, 2012, 32(10):2461-2469 Han J C, Bi C J, Chen Z L, et al. Pollution characteristics of PAHs in urban runoffs from main roads in urban area[J]. Acta Scientiae Circumstantiae, 2012, 32(10):2461-2469(in Chinese)
郭娉婷.生物滞留设施生态水文效应研究[D].北京:北京建筑大学, 2015:32-36 Guo P T. Eco-hydrological effects of bioretention facility[D]. Beijing:Beijing University of Civil Engineering and Architecture, 2015:32 -36(in Chinese)
王佳,王思思,车伍,等.雨水花园植物的选择与设计[J].北方园艺, 2012, 1(19):77-81 Wang J, Wang S S, Che W, et al. Plant selection and design of rain garden[J]. Northern Horticulture, 2012, 1(19):77-81(in Chinese)
罗红梅,车伍,李俊奇,等.雨水花园在雨洪控制与利用中的应用[J].中国给水排水, 2008, 24(6):48-52 Luo H M, Che W, Li J Q, et al. Application of rainwater garden to storm and flood control and utilization[J]. China Water & Wastewater, 2008, 24(6):48-52(in Chinese)
刘燕,尹澄清,车伍.植草沟在城市面源污染控制系统的应用[J].环境工程学报, 2008, 2(3):334-339 Liu Y, Yin C Q, Che W. Application of grassed swales in urban non-point source pollution control[J]. Chinese Journal of Environmental Engineering, 2008, 2(3):334-339(in Chinese)
曹治国,王萌萌,王小颍,等.办公室地面灰尘中PAHs污染的时间变化规律及人体健康风险[J].生态毒理学报, 2018, 13(3):209-219 Cao Z G, Wang M M, Wang X Y, et al. Time variation of polycyclic aromatic hydrocarbons in floor dust from office and corresponding human health risks[J]. Asian Journal of Ecotoxicology, 2018, 13(3):209-219(in Chinese)
Palla A, Gnecco I, Lanza L G. Unsaturated 2D modeling of subsurface water flow in the coarse-grained porous matrix of a green roof[J]. Journal of Hydrology, 2009, 379(1):193-204 Werthmann C. Green Roof:A Case Study[M]. New York:Princton Architectural Press, 2007:35-38 -
点击查看大图
计量
- 文章访问数: 1708
- HTML全文浏览数: 1708
- PDF下载数: 29
- 施引文献: 0
下载:
